激光点阵扫描法绝对定标太阳辐射计直射通道研究

利用可调谐激光器作为光源,以溯源于低温绝对辐射计的标准传递探测器作为激光束功率测量探测器,采用激光点阵扫描方法在太阳辐射计有效孔径光阑面形成均匀照度场,精确测量太阳辐射计870 nm无偏直射通道中心波长处绝对辐照度响应度。利用灯-单色仪系统扫描获得该通道相对光谱辐照度响应度,最终在实验室条件下获得该通道绝对光谱辐照度响应度,联合大气层外太阳照度谱数据通道内积分得到该通道大气层外响应常数V₀值,与NASA的GSFC中心的2009年定标结果差异仅为3.75%,定标不确定度达到2.06%,验证了这一新技术的原理可行性。     

Insights into the Time Evolution of Slowly Photodegrading Contaminants

Photochemical degradation plays an important role in the attenuation of many recalcitrant pollutants in surface freshwaters. Photoinduced transformation kinetics are strongly affected by environmental conditions, where sunlight irradiance plays the main role, followed by water depth and dissolved organic carbon (DOC). Apart from poorly predictable weather-related issues, fair-weather irradiance has a seasonal trend that results in the fastest photodegradation in June and the slowest in December (at least in temperate areas of the northern hemisphere). Pollutants that have first-order photochemical lifetimes longer than a week take more than one month to achieve 95% photodegradation. Consequently, they may experience quite different irradiance conditions as their photodegradation goes on. The relevant time trend can be approximated as a series of first-order kinetic tracts, each lasting for one month. The trend considerably departs from an overall exponential decay, if degradation takes long enough to encompass seasonally varying irradiance conditions. For instance, sunlight irradiance is higher in July than in April, but increasing irradiance after April and decreasing irradiance after July ensure that pollutants emitted in either month undergo degradation with very similar time trends in the first 3–4 months after emission. If photodegradation takes longer, pollutants emitted in July experience a considerable slowdown in photoreaction kinetics as winter is approached. Therefore, if pollutants are photostable enough that their photochemical time trend evolves over different seasons, degradation acquires some peculiar features than cannot be easily predicted from a mere analysis of lifetimes in the framework of simple first-order kinetics. Such features are here highlighted with a modelling approach, taking the case of carbamazepine as the main example. This contaminant is almost totally biorecalcitrant, and it is also quite resistant to photodegradation.     

基于探测器标准的高精度光谱辐射标准光源

本文在评述低温绝对辐射计和SIRCUS发展的基础上,讨论了基于探测器标准的光谱可调谐自校准标准光源的工作原理、发展与应用前景。在探测器型光谱辐射标准研究方面,工作在液氦温度的低温绝对辐射计不确定度达0.01%。美国国家标准与技术研究院(NIST)建立的均匀光源光谱辐照度和光谱辐亮度响应度定标装置(SIRCUS)采用一系列激光器,由低温绝对辐射计传递的硅陷阱探测器定标,不确定度已达到0.1%,成功应用于空间遥感仪器高精度辐射定标。分析认为,发展中的基于探测器标准的光谱可调谐自校准标准光源,定标精度高,自行校正老化、衰减,保证了定标精度长期稳定。     

氙灯光源太阳模拟器辐照衰减器设计方法

针对应用于太阳模拟器辐照衰减器设计上的不足,提出一种新的衰减器设计方法,旨在提高其辐照均匀性。基于光学扩展量计算衰减器上的网孔面积,对会聚光路的辐射通量进行调制;利用聚光镜环带法,理论上分析衰减器上的辐射分布;利用网孔非均匀分布的结构对会聚光路的辐射分布进行调制,给出具体设计参数;对比分析了网孔均匀分布和非均匀分布对辐射调制效果和辐照均匀性的影响。实验表明:安装网孔非均匀分布的衰减器,调节氙灯功率,能够连续输出0.1~1.0个太阳常数的辐照度;基于网孔非均匀分布的衰减器对辐射分布调制后,光斑内辐照不均匀度降低率最高为48.7%,低辐照不均匀度下可以实现辐照度的大范围调整,对提高太阳模拟器的使用性能具有一定的借鉴意义。     

利用光强分布转换器件实现低能耗光学超分辨

依据基模（ＴＥＭ００）高斯光束本身的横向光强分布,结合一类光强分布转换器件的转换特性,提出一种衫型低能耗光学超分辨的新方案,高斯光中央峰入射这类器件后,将从器件的边缘出射,而入射到边缘的光则从中央出射,由此,在成像系统中就可实现光学超分辨,与原有的滤波器比较,大大降低了能量的损耗。     

Classification of rough surfaces: comparison between two hybrid optical coherent processors

Two coherent optical approaches to the classification of rough surfaces using Fourier techniques are compared. Results for various machined metal samples show the potentials of these non-destructive techniques for roughnesses of R_t ranging from 0.1 to 10 μm.     

二元环形孔径全空间轴线上的衍射光强分布

运用Rayleigh-Sommerfeld衍射积分,详细推导了二元环形孔径全空间在轴光强分布公式.由于未作明显的近似,所得公式对衍射距离大于数倍入射波长的衍射空间都是有效的.计算并分析了这种孔径轴线上的光强分布情况.结果显示,它的最大调制深度是入射光强的16倍,比圆形孔径或环形孔径大4倍,近场的光学层析能力比远场的强.在很近场区,二元环形孔径的在轴光强分布对孔径结构比较敏感,这些特性使这种孔径在光子学和光纤光学的应用方面具有潜在的价值.     

The acclimative response of the main light-harvesting chlorophyll a/b-protein complex of photosystem II (LHCII) to elevated irradiances at the level of trimeric subunits

The changes in structural organization of the major light-harvesting chlorophyll a/b–protein complex of photosystem II (LHC II) at the level of trimeric subcomplexes were studied in spinach plants grown under low light conditions (50 μmol quanta m⁻² s⁻¹) and then acclimated to elevated irradiances. By monitoring photochemical quenching of fluorescence yield (q_P), photosystem II (PS II) functional status was assessed in leaves of plants acclimated to a range of elevated irradiances. Three separate acclimative irradiances were selected for the experiments, reflecting: limiting light conditions (150 μmol quanta m⁻² s⁻¹), near to the inflexion point on the irradiance curve conditions (300 μmol quanta m⁻² s⁻¹) and an excessive light, causing a moderate stress in the form of down regulation of PS II (450 μmol quanta m⁻² s⁻¹). An immunoblot analysis showed that there was a clear decline in an abundance on chlorophyll basis of Lhcb1-3 apoproteins as an acclimative irradiance increased from 50 to 450 μmol quanta m⁻² s⁻¹, with Lhcb1 decreasing to a lesser extent than Lhcb2 and Lhcb3 (only at excessive irradiance). When analyzed by non-denaturing isoelectric focusing BBY membrane fragments (PSII-enriched, stacked thylakoid membranes) isolated from low light-grown plants were resolved into nine fractions, seven of which (labelled 3–9) were established by us previously [Jackowski and Pielucha, J. Photochem. Photobiol. B: Biol. 64 (2001) 45] to be LHC II subcomplexes representing mixed populations of closely similar trimers, comprising permutations of Lhcb1 and Lhcb2 (subcomplexes 3–7) or Lhcb1-3 (subcomplexes 8 and 9). A heterogeneity with regard to accumulation behaviour of LHC II subcomplexes in response to elevated irradiances was revealed. The subcomplexes 5 and 6 were accumulating at similar level, regardless of the light irradiance experienced. Another group consisting of the subcomplexes 3 and 4 (the most basic ones) showed a progressive increase in relative abundance with increasing an irradiance intensity whereas the subcomplexes 7–9 (the most acidic ones) exhibited a progressive decline in their relative abundance during an acclimation of spinach plants to elevated irradiances thus they may collectively represent an elevated irradiance-responsive subunit of LHCII.     

Transient photocapacitance study in 4-nitro-4′-aminodiphenyl layers

In 4-nitro-4-aminodiphenyl (NAD) layers the photocapacitance (PhC) transients were investigated. PhC spectral distribution as well as the temperature dependences of time constants (under/_on/or after/_off/illumination) have been measured. The photocapacitance spectral distribution possesses maxima at 350, 500, and 750 nm. It was shown that _on (T) is of exponential form while _off (T) is more complicated. The values of thermal activation energies (0.65±0.05) eV of both time constants coincide. The mechanism of photocapacitance process has been disclosed in NAD layers.     

DEUTERIUM INFLUX PROFILE ALONG THE APEX OF THE UPPER X-POINT TILES IN JET

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